A Link Between Worlds would be a safe bet. For future consideration, play Ocarina of Time 3D if you haven't yet. Also, for future consideration, the Legend of Zelda games on the DS were good, those were Phantom Hourglass and Spirit Tracks.
If you love JRPGs, I'd consider the Shin Megami Tensei games, which there's a good deal of on the 3DS, they have Devil Survivor: Overlocked (remake of the DS game) and Devil Survivor 2: Record Break coming (also a remake of the DS version), Soul Hackers, a remake of an older Saturn game, actualy fun, and SMT4, which was originally designed for the 3DS, and of course Persona Q which is coming in November. Keep in mind you can also play DS games, so there's the option of SMT: Strange Journey, and of course Devil Survivor 2 which hasn't been upgraded for the 3DS yet (and who knows when that'll happen, was supposed to be last year). And of course, with Persona Q coming out, if you're considering it I'd dabble in some Persona 3 and 4 if you haven't already to bring yourself up to speed (and that by itself is its own reward)... that's on PS2 though, but if you have a PS3 I believe they're on the PS Store, along with other classic SMT games.
If you're into Phoenix Wright and/or Professor Layton games, the crossover game is coming out next week. And if not the Phoenix Wright Ace Attorney Trilogy should be releasing soon.
Oh, if you haven't tried Luigi's Mansion Dark Moon yet, you should... at some point.
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