Catherine and Nier Automata were pretty unique, though I didn't enjoy those games much.
Crazy Taxi was kind of unique. I bought it for Dreamcast and thought I would have a fun but very short arcade-like experience. But I found out it had exceptionally deep gameplay.
A lot of other games were unique when they first came out. Here are a few on top of my head.
Double Dragon (Arcade). First scrolling beat'em'up which had a lot of interesting weapons to pick up, and you could climb up ladders. Wow!
Wipeout (PS1). First time we experienced amazingly fast 3D spacecraft racing.
Exploding Fist 2 (C64). A scrolling beat'em'up consisting of more than 100 screens. Revolutionary at its time.
Larry 1. The first RPG game with the objective to bang women.
Bioshock. The world felt so unique.
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