I'll second DotA 2 and LoL. Most of the community in those games are extremely stupid and easily agitated. Stuff like picking wrong heroes, wrong items, pretending that you don't speak english and etc. can make the other players go into a frenzy. In DotA there is the addes bonus of trolling through voice chat as well as picking certain heroes and using their abilities to troll your allies (teleporting them inside impasable terrain or to the enemy base and etc,)
You can troll/grief in most MMORPGs that have open pvp. Just repeatedly gank people who are questing and you're sure to stir up some reaction.
Also, games like counterstrike - voice chat trolling, killing your own team, all that stuff.
Personally I've had the most fun trolling a MMORPG called Runes of Magic because it had easily abusable mechanics but right now the game is quite dead.
But I think you'll have the most success making people mad in DotA 2 and LoL.
One more thing I forgot to add - LoL has a game mode called 'Ranked'. It requires some grinding to get access to it, but once you can you can do some quality trolling. The people playing ranked get mad (like really MAD) over the stupidest, inconsequential things. Often you don't even need to try to make them angry.
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