In no particular order-
1. Team Fortress 2
2. Counter-Strike: Source (Or 1.6)
3. The Witcher
4. Crysis
5. Battlefield 2
6. Diablo 2
7. Fallout 3
8. Deux Ex
9. ARMA 2
10. Warcraft III
And if you're into MMO's, some good ones to try are WoW, Aion, or AoC.
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