i second the recommended games...
crayon physics deluxe, braid, world of goo, multiwinia, gravitron 2...
and here are a few excellent free games
gravity bone (fantastic polished stylish first person secret agent adventure...great short experiecne.about 20 min to finish)
http://www.blendogames.com/
phun (sandbox game)
http://www.phunland.com/wiki/Home
bontago (block building physic based startegythathas also a sandbox mode)
http://www.bontago.com/
flywrench (abstract fun! control a flying wrench)
http://www.messhof.com/games/flywrench.php
neverball (monkey ball clone)
http://neverball.org/
typogun (arcade typing game...typing and shooting)
http://pondspark.blogspot.com/2001/01/typogun_9514.html
strange attractors 1 (great one switch game...)
http://www.ominousdev.com/games.php
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