Wii. It's fully backwards compatible with the GC, which was the only system with RE0. Therefore, you can play all of the other RE games without any trouble, not to mention it's about 1000x easier to find component cables for it than the GC. Also, with the Wii re-releases of RE0 and 1 it's a bit easier to find them... 2 and 3 for GC are rather difficult to find (these are ports of the Dreamcast versions, which had higher resolution than the PS1 versions), but Code Veronica X is worth searching for on GC because it's the best version that released outside of Japan.
Also, the Wii has the best version of RE4 (better graphics and sound of the GC version, new content of the PS2/PC version, and a few others tweaks to the weapons and characters that improve it further, along with the control scheme), and it's the only way you can play Umbrella Chronicles (fills in the gaps between the games).
Know that your PS1 is already backwards compatible with PS1 games though... if you can't find the GC versions of RE2 and 3, there's nothing wrong with getting them on there. However, if you're looking to have all of the main series RE games pre-5 on one system, the GC and Wii are your only options.
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