Devil May Cry 4: Credo. "I am an angel!!!" Best boss fight the game has to offer. Very climatic, lots of cool quotes, not too easy and that guy just looks way too kick-ass.
Tales of Vesperia: This game has a lot really cool and climatic boss fights. Best ones are by far the fights against Schwann and Alexei. The characters itself stand out so much, it feels really great being finally able to fight them. Also the Schwann fight starts with a very big surprise which makes you wonder if you are even supposed to bring him down or not.
No More Heroes 2: Margaret, "Reaper, reaper, thats what people call me..." Addicting song, stylish boss, cool fight. My favourite assassin of the series.
Resident Evil 4: Krauser (especially the quick-time knife fight is extremely epic)
Resident Evil 5: Wesker (again the quick time event in the plane is my favourite part of that boss)
Tales of Graces: First Richard fight. Very, very, very climatic and emotional, not to mention the superb anime sequence after the fight. The high point of the game.
Tales of the Abyss: First Asch fight, final Asch fight, final boss, I am able to ingore the flaws of this game if I think back to these fights.
Tales of Symphonia: First time you enter the Tower of Salvation, very entertaining bosses await you.
Dawn of the New World: Second Richter fight was really cool, but this game also has a lot of cool bosses.
Kingdom Hearts 2: Every boss the final dungeon has to offer. This is the reason why I love this game, yeah its mostly because of the final dungeon. xD
Eternal Sonata: All Fugue fights. I love that guy.
Yeah I could go on, but this is the best of the best in my opinion.
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