It would help to know what kind of games you like. But Guild Wars 2, The Witcher 1&2, XCOM: Enemy Unkown, Civ V are all excellent just to get started...
On a more serious note: Imo Mass Effect 1 is more fun on the consoles but it is by no means bad on the PC. Its just the controls are far more awkward. And the minigame in that vers is annoying as hell. And there are far more technical issues. Also I'll second the Witcher 2 recommendation. Might also want to give the dragon age series a try if you haven't already.
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